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I haven't found a pattern here. It occurs with some FLAC files I receive from friends and some I rip myself using Max. It doesn't occur too often, and I've seemed to resolve it for most of the files I rip myself by using compression level 6 instead of the default of 5 in Max. But now I've tried both ripping and downloading a FLAC of Rush' Tom Sawyer and it consistently crashes iTunes no matter what settings I use while ripping. Still it plays fine in QuickTime player (and throug Finder previews).

I'll attach a text file with the most recent crash log which also indicates my OS and iTunes version.

(I could also add that the rest of the album Moving Pictures by Rush plays fine, heh.)